A nitrogen-doped carbon-coated silicon carbide as a robust and highly efficient metal-free catalyst for sour gas desulfurization in the presence of aromatics as contaminants

Author:

Duong-Viet Cuong12345,Nhut Jean-Mario12345,Truong-Huu Tri6789,Tuci Giulia10111213,Nguyen-Dinh Lam6789,Liu Yuefeng14151617ORCID,Pham Charlotte181920,Giambastiani Giuliano12345ORCID,Pham-Huu Cuong12345

Affiliation:

1. Institute of Chemistry and Processes for Energy

2. Environment and Health (ICPEES)

3. UMR 7515 CNRS

4. Université de Strasbourg

5. 67087 Strasbourg Cedex 02

6. The University of Da-Nang

7. University of Science and Technology

8. Da-Nang

9. Vietnam

10. Institute of Chemistry of OrganoMetallic Compounds

11. ICCOM-CNR and Consorzio INSTM

12. Florence

13. Italy

14. Dalian National Laboratory for Clean Energy (DNL)

15. Dalian Institute of Chemical Physics, Chinese Academy of Science

16. 116023 Dalian

17. China

18. SICAT SARL

19. 67000 Strasbourg

20. France

Abstract

A mesoporous N-doped carbon coating for SiC extrudates shows excellent H2S desulfurization performance along with remarkably high resistance towards deactivation/fouling in the presence of aromatics as contaminant.

Funder

Agence Nationale de la Recherche

National Natural Science Foundation of China

Ministero dell’Istruzione, dell’Università e della Ricerca

National Foundation for Science and Technology Development

Youth Innovation Promotion Association of the Chinese Academy of Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

Catalysis

Reference73 articles.

1. (last access 28/04/ 2020 ), https://www.ucsusa.org/resources/uses-natural-gas

2. (last access 28/04/ 2020 ), https://www.swarthmore.edu/environmental-studies-capstone/comparison-against-other-fossil-fuels

3. Catalytic and adsorptive desulphurization of gases

4. Recovery of sulfur from sour acid gas: A review of the technology

5. Claus Catalysis and H2S Selective Oxidation

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