Copper-catalyzed amine-mediated yne-propargylic substitution

Author:

Jiang Chunyun1,Luo Defu1,Meng Xiangjian2,Cui Qinqin3,Zhao Lili4,Liu Jinggong5ORCID,Yang Shuang4,Fang Xinqiang14ORCID

Affiliation:

1. College of Chemistry, Fuzhou University, Fuzhou 350116, China

2. Fujian Normal University, Fuzhou 350108, China

3. School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832000, China

4. State Key Laboratory of Structural Chemistry, Center for Excellence in Molecular Synthesis, Fujian Institute of Research on the Structure of Matter, University of Chinese Academy of Sciences, Fuzhou 350100, China

5. Orthopedics Department, Guangdong Provincial Hospital of Traditional Chinese Medicine, The Second Affiliated Hospital of Guangzhou University of Chinese Medicine, Guangzhou 510120, China

Abstract

A copper-catalyzed yne-propargylic substitution using amines as nucleophiles has been achieved for the first time, affording a variety of amines having diyne moieties, which are important pharmacophores in many bioactive molecules.

Funder

National Natural Science Foundation of China

Chinese Academy of Sciences

Natural Science Foundation of Fujian Province

Publisher

Royal Society of Chemistry (RSC)

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