Three-photon-induced singlet excited-state absorption for tunable ultrafast optical-limiting in distyrylbenzene: a first-principles study

Author:

Zhang Danyang1,Zhu Hongjuan1,Wang Chunrui2,Kang Shuying3,Zhou Yong1ORCID,Sheng Xiaowei1ORCID

Affiliation:

1. Anhui Province Key Laboratory of Optoelectric Materials Science and Technology, Department of Physics, Anhui Normal University, Anhui, Wuhu 241000, China

2. State Key Laboratory of Laser Interaction with Matter, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Science, Changchun 130033, China

3. School of Physics and Electronic Information, Gannan Normal University, Ganzhou 341000, China

Abstract

The present paper illustrates that distyrylbenzene is a promising ultrafast optical limiter for wavelengths around 775 nm, which can be well understood by three-photon induced excited state absorption.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Anhui Province

Hefei Science Center, Chinese Academy of Sciences

State Key Laboratory of Laser Interaction with Matter

Youth Innovation Promotion Association

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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