Novel hydrogen chemisorption properties of amorphous ceramic compounds consisting of p-block elements: exploring Lewis acid–base Al–N pair sites formed in situ within polymer-derived silicon–aluminum–nitrogen-based systems-Reference-Cited by-同舟云学术

Novel hydrogen chemisorption properties of amorphous ceramic compounds consisting of p-block elements: exploring Lewis acid–base Al–N pair sites formed in situ within polymer-derived silicon–aluminum–nitrogen-based systems

Published:2021 Issue:5 Volume:9 Page:2959-2969
ISSN:2050-7488
Container-title:Journal of Materials Chemistry A
language:en
Short-container-title:J. Mater. Chem. A

Author:

Tada Shotaro¹²³⁴⁵^ORCID,Asakuma Norifumi¹²³⁴⁵,Ando Shiori¹²³⁴⁵,Asaka Toru¹²³⁴⁵,Daiko Yusuke¹²³⁴⁵^ORCID,Honda Sawao¹²³⁴⁵,Haneda Masaaki¹²³⁴⁵^ORCID,Bernard Samuel⁶⁷⁸⁹¹⁰^ORCID,Riedel Ralf¹¹¹²¹³¹⁴,Iwamoto Yuji¹²³⁴⁵^ORCID

Affiliation:

1. Department of Life Science and Applied Chemistry

2. Graduate School of Engineering

3. Nagoya Institute of Technology

4. Nagoya 466-8555

5. Japan

6. University of Limoges

7. CNRS

8. IRCER

9. UMR 7315

10. Limoges

11. Institut für Materialwissenschaft

12. Technische Universität Darmstadt

13. 64287 Darmstadt

14. Germany

Abstract

This paper reports the relationship between the H₂ chemisorption properties and reversible structural reorientation of the possible active sites around Al formed in situ within polymer-derived ceramics (PDCs) based on an amorphous Si–Al–N system.

Funder

Centre National de la Recherche Scientifique

Japan Society for the Promotion of Science

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2021/TA/D0TA10271G

Reference44 articles.

1. Selective Hydrogenation over Supported Metal Catalysts: From Nanoparticles to Single Atoms

2. The Surface Chemistry of Metal-Based Hydrogenation Catalysis