Transition from antiferromagnetic ground state to robust ferrimagnetic order with Curie temperatures above 420 K in manganese-based antiperovskite-type structures

Author:

Zhang Xinghong1234,Yuan Quan1234,Gao Tangling5674,Ren Yang89101112ORCID,Wu Hui13141512ORCID,Huang Qingzhen13141512,Zhao Jinggeng1623417ORCID,Wang Xianjie16234,Yuan Ye1819202122,Xu Chi1819202122,Hu Yongfeng232425,Dynes James J.232425,Zhou Jigang232425ORCID,Zhou Shengqiang18192021,Liu Yu1819202126,Song Bo123416ORCID

Affiliation:

1. Center for Composite Materials and Structures

2. Harbin Institute of Technology

3. Harbin 150001

4. China

5. Institute of Petrochemistry

6. Heilongjiang Academy of Sciences

7. Harbin 150040

8. X-Ray Science Division

9. Advanced Photon Source

10. Argonne National Laboratory

11. Argonne

12. USA

13. NIST Center for Neutron Research

14. National Institute of Standards and Technology

15. Gaithersburg

16. Department of Physics

17. Academy of Fundamental and Interdisciplinary Sciences

18. Helmholtz-Zentrum Dresden-Rossendorf

19. Institute of Ion Beam Physics and Materials Research

20. 01328 Dresden

21. Germany

22. Technische Universität Dresden

23. Canadian Light Source Inc.

24. Saskatoon

25. Canada

26. Center for Quantum Devices

Abstract

Robust ferrimagnetic order is found in Mn3GaxNx when x = 0.5, 0.6, and 0.7 with Curie temperature in the range of ∼390–420 K.

Funder

National Natural Science Foundation of China

Program for New Century Excellent Talents in University

Natural Science Foundation of Heilongjiang Province

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,General Chemistry

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