A designed second-sphere hydrogen-bond interaction that critically influences the O–O bond activation for heterolytic cleavage in ferric iron–porphyrin complexes-Reference-Cited by-同舟云学术

A designed second-sphere hydrogen-bond interaction that critically influences the O–O bond activation for heterolytic cleavage in ferric iron–porphyrin complexes

Published:2020 Issue:10 Volume:11 Page:2681-2695
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Bhunia Sarmistha¹²³⁴^ORCID,Rana Atanu¹²³⁴^ORCID,Dey Somdatta Ghosh¹²³⁴^ORCID,Ivancich Anabella⁵⁶⁷⁸⁹^ORCID,Dey Abhishek¹²³⁴^ORCID

Affiliation:

1. Department of Inorganic Chemistry

2. Indian Association for the Cultivation of Science

3. Kolkata

4. India

5. CNRS

6. Aix-Marseille Univ

7. Laboratoire de Bioénergétique et Ingénierie des Protéines (UMR 7281)

8. IMM FR3479

9. Marseille

Abstract

Heme hydroperoxidases catalyze the oxidation of substrates by H₂O₂.

Funder

Science and Engineering Research Board

Department of Science and Technology, Ministry of Science and Technology

Council of Scientific and Industrial Research, India

Centre National de la Recherche Scientifique

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2020/SC/C9SC04388H

Reference90 articles.

1. Factors Determining the Rate and Selectivity of 4e–/4H+ Electrocatalytic Reduction of Dioxygen by Iron Porphyrin Complexes

2. Critical Aspects of Heme–Peroxo–Cu Complex Structure and Nature of Proton Source Dictate Metal–Operoxo Breakage versus Reductive O–O Cleavage Chemistry

3. Intramolecular Hydrogen Bonding Enhances Stability and Reactivity of Mononuclear Cupric Superoxide Complexes

4. Peroxo and Superoxo Moieties Bound to Copper Ion: Electron-Transfer Equilibrium with a Small Reorganization Energy

5. Selective Formation of an FeIV O or an FeIII OOH Intermediate From Iron(II) and H2 O2 : Controlled Heterolytic versus Homolytic Oxygen-Oxygen Bond Cleavage by the Second Coordination Sphere

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