Green and alcohol-free H2O2 generation paired with simultaneous contaminant treatment enabled by sulfur/cyano-modified g-C3N4 with efficient oxygen activation and proton adsorption

Author:

Wang Zijie1,Wu Jiaqi1,Fan Xiaoqiong1,Zhang Yiwen1,Xu Qing1,Qiu Bocheng2ORCID,Chen Liang1,Zeng Xiaofei1ORCID,Zhu Qiaohong1

Affiliation:

1. College of Material, Chemistry and Chemical Engineering, Key Laboratory of Organosilicon Chemistry and Material Technology, Ministry of Education, Hangzhou Normal University, Hangzhou, 311121, Zhejiang, China

2. Jiangsu Key Laboratory of Pesticide Sciences, Department of Chemistry, College of Sciences, Nanjing Agricultural University, Nanjing 210095, China

Abstract

A S atom and cyano group co-modified carbon nitride was synthesized for alcohol-free H2O2 generation paired with simultaneous contaminant treatment. S atoms facilitate oxygen adsorption and cyano groups lead to the promotion of H+ adsorption.

Funder

Natural Science Foundation of Zhejiang Province

National Natural Science Foundation of China

Hangzhou Normal University

Publisher

Royal Society of Chemistry (RSC)

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