Boosting the turnover number of core–shell Al-ZSM-5@B-ZSM-5 zeolite for methanol to propylene reaction by modulating its gradient acid site distribution and low consumption diffusion
Author:
Affiliation:
1. State Key Laboratory of Heavy Oil Processing and the Key Laboratory of Catalysis of CNPC
2. China University of Petroleum
3. Beijing 102249
4. China
5. Wuhan Institute of Physics and Mathematics
6. Chinese Academy of Sciences
7. Wuhan 430071
Abstract
Hierarchical Al-ZSM-5@B-ZSM-5 core–shell zeolite was prepared to boost turnover number of MTP reaction.
Funder
National Natural Science Foundation of China
Publisher
Royal Society of Chemistry (RSC)
Subject
Catalysis
Link
http://pubs.rsc.org/en/content/articlepdf/2019/CY/C8CY02177E
Reference60 articles.
1. Selective production of propylene from methanol: Mesoporosity development in high silica HZSM-5
2. The formation and degradation of active species during methanol conversion over protonated zeotype catalysts
3. Conversion of Methanol into Hydrocarbons over Zeolite H-ZSM-5: Ethene Formation Is Mechanistically Separated from the Formation of Higher Alkenes
4. A mechanistic basis for the effects of crystallite size on light olefin selectivity in methanol-to-hydrocarbons conversion on MFI
5. Facile fabrication of mesopore-containing ZSM-5 zeolite from spent zeolite catalyst for methanol to propylene reaction
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