New insights into the NH3-selective catalytic reduction of NO over Cu-ZSM-5 as revealed by operando spectroscopy

Author:

Ye Xinwei12ORCID,Oord Ramon2ORCID,Monai Matteo2,Schmidt Joel E.2,Chen Tiehong1ORCID,Meirer Florian2,Weckhuysen Bert M.2ORCID

Affiliation:

1. Institute of New Catalytic Materials Science, School of Materials Science and Engineering, Key Laboratory of Advanced Energy Materials Chemistry (MOE), Nankai University, Tianjin 300350, China

2. Inorganic Chemistry and Catalysis Group, Debye Institute for Nanomaterials Science, Utrecht University, Universiteitsweg 99, 3584 CG Utrecht, The Netherlands

Abstract

To control diesel vehicle NOx emissions, Cu-exchanged zeolites have been applied in the selective catalytic reduction of NO using NH3 as reductant. In this work, the local structure of Cu2+ in zeolite ZSM-5 has been revealed by operando spectroscopies.

Funder

Nederlandse Organisatie voor Wetenschappelijk Onderzoek

China Scholarship Council

Publisher

Royal Society of Chemistry (RSC)

Subject

Catalysis

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