Understanding ring-closing and racemization to prepare α-amino acid NCA and NTA monomers: a DFT study-Reference-Cited by-同舟云学术

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Understanding ring-closing and racemization to prepare α-amino acid NCA and NTA monomers: a DFT study

Published:2020 Issue:26 Volume:22 Page:14868-14874
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Bai Tianwen¹²³⁴⁵,Shen Bo⁶⁷³⁸⁵,Cai Da⁶⁷³⁸⁵,Luo Yifan⁶⁹¹⁰⁵,Zhou Peng¹²³⁴⁵,Xia Jingya⁶⁷³⁸⁵,Zheng Botuo¹²³⁴⁵,Zhang Ke⁶⁷³⁸⁵,Xie Rongze⁶¹¹¹²⁵,Ni Xufeng¹²³⁴⁵,Xu Maosheng⁶⁹¹⁰⁵,Ling Jun¹²³⁴⁵^ORCID,Sun Jihong⁶⁷³⁸⁵

Affiliation:

1. MOE Key Laboratory of Macromolecular Synthesis and Functionalization

2. Department of Polymer Science and Engineering

3. Zhejiang University

4. Hangzhou 310027

5. China

6. Department of Radiology

7. Sir Run Run Shaw Hospital

8. Hangzhou 310016

9. The First Affiliated Hospital of Zhejiang Chinese Medical University

10. Hangzhou

11. Jiulongpo People's Hospital

12. Chongqing 400050

Abstract

Our work demonstrates the detailed mechanism to synthesize NCA and NTA monomers and racemization process of optical pure monomers.

Funder

National Natural Science Foundation of China

National Basic Research Program of China

Natural Science Foundation of Shaanxi Province

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

Link

http://pubs.rsc.org/en/content/articlepdf/2020/CP/D0CP01174F

Reference37 articles.

1. Polysarcosine-containing copolymers: Synthesis, characterization, self-assembly, and applications

2. Star-Shaped Polypeptides: Synthesis and Opportunities for Delivery of Therapeutics

3. Peptoids and Polypeptoids at the Frontier of Supra- and Macromolecular Engineering

4. Sequence Programmable Peptoid Polymers for Diverse Materials Applications

5. Recent advances in glycopolypeptide synthesis

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1. An Inspection into Multifarious Ways to Synthesize Poly(Amino Acid)s;Macromolecular Rapid Communications;2021-10-13

2. Telechelic Triblock Poly( α‐Amino Acid)‐Poly(Tetrahydrofuran)‐Poly( α‐Amino Acid) Copolymers: Chain‐End Transformation, Polymerization and pH‐Responsive Hydrolysis †;Chinese Journal of Chemistry;2021-08-15

3. Ring-Opening Polymerization of CO2-Based Disubstituted δ-Valerolactone toward Sustainable Functional Polyesters;ACS Macro Letters;2021-07-29

4. Density Functional Theory Studies on the Synthesis of Poly(α-Amino Acid)s Via the Amine-Mediated Ring Opening Polymerizations of N-Carboxyanhydrides and N-Thiocarboxyanhydrides;Frontiers in Chemistry;2021-03-29

5. Synthesis of Well-defined Poly(tetrahydrofuran)-b-Poly(a-amino acid)s via Cationic Ring-opening Polymerization (ROP) of Tetrahydrofuran and Nucleophilic ROP of N-thiocarboxyanhydrides;Chinese Journal of Polymer Science;2021-01-05

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