Entropy stabilized cubic Li7La3Zr2O12 with reduced lithium diffusion activation energy: studied using solid-state NMR spectroscopy-Reference-Cited by-同舟云学术

Entropy stabilized cubic Li₇La₃Zr₂O₁₂ with reduced lithium diffusion activation energy: studied using solid-state NMR spectroscopy

Published:2023 Issue:29 Volume:13 Page:19856-19861
ISSN:2046-2069
Container-title:RSC Advances
language:en
Short-container-title:RSC Adv.

Author:

Fan Juntian¹²,Wang Tao²,Bridges Craig A.²,Borisevich Albina Y.³^ORCID,Steren Carlos A.¹^ORCID,Li Pengzhen⁴,Thapaliya Bishnu P.²,Do-Thanh Chi-Linh¹^ORCID,Yang Zhenzhen²,Yuan Yating²,Dai Sheng¹²^ORCID

Affiliation:

1. Department of Chemistry, University of Tennessee, Knoxville, TN 37996, USA

2. Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, 37831, USA

3. Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, 37831, USA

4. Department of Agricultural and Resource Economics, University of Tennessee, Knoxville, TN 37996, USA

Abstract

A high-entropy strategy at Zr sites was achieved to stabilize cubic Li7La3Zr2O12 and reduce lithium diffusion activation energy, demonstrated by SSNMR.

Funder

U.S. Department of Energy

Office of Science

Basic Energy Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemical Engineering,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2023/RA/D3RA02206D

Reference37 articles.

1. Fundamentals of inorganic solid-state electrolytes for batteries

2. Lithium battery chemistries enabled by solid-state electrolytes

3. Fast Lithium Ion Conduction in Garnet-Type Li7La3Zr2O12

4. Recent Advances in Energy Chemistry between Solid-State Electrolyte and Safe Lithium-Metal Anodes

5. Challenges and perspectives of garnet solid electrolytes for all solid-state lithium batteries

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