Direct observation of DME carbonylation in the different channels of H-MOR zeolite by continuous-flow solid-state NMR spectroscopy-Reference-Cited by-同舟云学术

Direct observation of DME carbonylation in the different channels of H-MOR zeolite by continuous-flow solid-state NMR spectroscopy

Published:2015 Issue:94 Volume:51 Page:16868-16870
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

He Ting¹²³⁴⁵,Ren Pengju¹²³⁴⁵,Liu Xianchun¹²³⁴⁵,Xu Shutao⁶⁷⁸³⁴,Han Xiuwen¹²³⁴⁵,Bao Xinhe¹²³⁴⁵

Affiliation:

1. State Key Laboratory of Catalysis

2. Dalian Institute of Chemical Physic

3. Chinese Academy of Sciences

4. Dalian 116023

5. P. R. China

6. National Engineering Laboratory for Methanol to Olefins

7. Dalian National Laboratory for Clean Energy

8. Dalian Institute of Chemical Physics

Abstract

Surface acetyl intermediates on HMOR zeolites (CH₃CO-Z) were detected during DME carbonylation using in situ continuous-flow ¹³C MAS NMR spectroscopy.

Funder

Ministry of Science and Technology of the People's Republic of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2015/CC/C5CC07201H

Reference20 articles.

1. High productivity methanol carbonylation catalysis using iridium

2. Selective Carbonylation of Dimethyl Ether to Methyl Acetate Catalyzed by Acidic Zeolites

3. Conversion of methanol to gasoline: new mechanism for formation of the first carbon-carbon bond

4. Methanol conversion on SAPO-34: reaction condition for fixed-bed reactor

5. Specificity of Sites within Eight-Membered Ring Zeolite Channels for Carbonylation of Methyls to Acetyls

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