Interfacial degradation of the NMC/Li6PS5Cl composite cathode in all-solid-state batteries

Author:

Hu Xudong1,Zhao Zishuo2,Zhao Yang1,Wang Xuelong3,Sainio Sami4,Nordlund Dennis4,Ruse Cristina M.5,Zhou Xiao-Dong5ORCID,Boettcher Shannon W.1ORCID,Hou Dong5,Hong Qi-Jun2,Mu Linqin2ORCID

Affiliation:

1. Department of Chemistry and Biochemistry, Oregon Center for Electrochemistry, University of Oregon, Eugene, OR 97403, USA

2. School for Engineering of Matter, Transport, and Energy, Arizona State University, Tempe, 85287, USA

3. Chemistry Division, Brookhaven National Laboratory, Upton, NY 11973, USA

4. Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA

5. Institute for Materials Research and Innovation (IMRI), University of Louisiana at Lafayette, Lafayette, LA 70503, USA

Abstract

Mitigating interfacial reactions in composite cathode materials remains a key challenge for high-performance all-solid-state batteries (ASSBs), particularly those employing argyrodite-based electrolytes coupled with high-voltage cathodes.

Funder

Arizona State University

Publisher

Royal Society of Chemistry (RSC)

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