A powder XRD, solid state NMR and calorimetric study of the phase evolution in mechanochemically synthesized dual cation (Csx(CH3NH3)1−x)PbX3 lead halide perovskite systems

Author:

Dintakurti Sai S. H.12ORCID,Walker David1ORCID,Bird Tobias A.3,Fang Yanan4ORCID,White Tim4,Hanna John V.14ORCID

Affiliation:

1. Department of Physics, University of Warwick, Coventry, West Midlands, CV4 7AL, UK

2. Interdisciplinary Graduate School, Nanyang Technological University, Singapore 639798, Singapore

3. Department of Chemistry, University of Warwick, Coventry, West Midlands, CV4 7AL, UK

4. School of Materials Science and Engineering, Nanyang Technological University, Singapore 639798, Singapore

Abstract

Mechanochemically synthesized dual cation hybrid perovskites of the form (CsxMA1−x)Pb(Cl/Br)3 (x = 0–1) exhibit complete miscibility and high structural order across each compositional range.

Funder

National Research Foundation Singapore

Science and Technology Facilities Council

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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