Co-photolysis of mixed chromophores affects atmospheric lifetimes of brown carbon

Author:

Wang Yalin1,Qiu Tian1,Zhang Cong1,Hao Tianwei1,Mabato Beatrix Rosette Go2,Zhang Ruifeng2,Gen Masao3,Chan Man Nin4ORCID,Huang Dan Dan5,Ge Xinlei6,Wang Junfeng6,Du Lin7ORCID,Huang Ru-Jin8,Chen Qi9,Hoi Ka In1,Mok Kai Meng1,Chan Chak K.210ORCID,Li Yong Jie1ORCID

Affiliation:

1. Department of Civil and Environmental Engineering, Department of Ocean Science and Technology, Centre for Regional Oceans, Faculty of Science and Technology, University of Macau, Macau 999078, China

2. School of Energy and Environment, City University of Hong Kong, Hong Kong 999077, China

3. Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, 2-1-1, Katahira, Sendai, Miyagi 980-8577, Japan

4. Earth System Science Programme, Faculty of Science, Institute of Environment, Energy, and Sustainability, The Chinese University of Hong Kong, Hong Kong 999077, China

5. Shanghai Academy of Environmental Sciences, Shanghai 200233, China

6. Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control (AEMPC), School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China

7. Environment Research Institute, Shandong University, Shanda South Road 27, Shandong 250100, China

8. State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China

9. State Key Joint Laboratory of Environmental Simulation and Pollution Control, BIC-ESAT, IJRC, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China

10. Physical Sciences and Engineering Division, King Abdullah University of Science and Technology, Kingdom of Saudi Arabia

Abstract

Sensitizing shortens the atmospheric lifetimes of BrC chromophores and potentially other species during (co-)photolysis, while shadowing only works in coarse particles.

Funder

Fundo para o Desenvolvimento das Ciências e da Tecnologia

Research Services and Knowledge Transfer Office, University of Macau

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry,Chemistry (miscellaneous),Analytical Chemistry

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