Operando sulfur speciation during sulfur poisoning-regeneration of Ru/SiO2 and Ru/Al2O3 using non-resonant sulfur Kα1,2 emission-Reference-Cited by-同舟云学术

Operando sulfur speciation during sulfur poisoning-regeneration of Ru/SiO2 and Ru/Al2O3 using non-resonant sulfur Kα1,2 emission

Published:2020 Issue:27 Volume:10 Page:15853-15859
ISSN:2046-2069
Container-title:RSC Advances
language:en
Short-container-title:RSC Adv.

Author:

Kuzmenko Dzulija¹²³⁴⁵^ORCID,Clark Adam H.¹²³^ORCID,Schildhauer Tilman¹²³,Szlachetko Jakub⁶⁷⁸⁹,Nachtegaal Maarten¹²³^ORCID

Affiliation:

1. Paul Scherrer Institut (PSI)

2. CH-5232 Villigen

3. Switzerland

4. Department of Chemistry and Applied Biosciences

5. ETH Zürich

6. Institute of Nuclear Physics

7. Polish Academy of Sciences

8. 31-342 Krakow

9. Poland

Abstract

Operando S Kα X-ray emission spectroscopy allows for a quantitative understanding of the sulfur poisoning and regeneration mechanism of state-of-the-art methanation catalysts used for the wood to synthetic natural gas process.

Funder

Narodowe Centrum Nauki

Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung

Energy System Integration, Paul Scherrer Institut

Innosuisse - Schweizerische Agentur für Innovationsförderung

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemical Engineering,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2020/RA/D0RA03068F

Reference18 articles.

1. T. J.Schildhauer , in Synthetic Natural Gas from Coal, Dry Biomass, and Power-to-Gas Applications , John Wiley & Sons, Ltd , 2016 , pp. 1–4

2. U.Rhyner , in Synthetic Natural Gas from Coal, Dry Biomass, and Power-to-Gas Applications , John Wiley & Sons, Ltd , 2016 , pp. 41–76

3. C. F. J.König , M.Nachtegaal and T. J.Schildhauer , in Synthetic Natural Gas from Coal, Dry Biomass, and Power-to-Gas Applications , John Wiley & Sons, Ltd , 2016 , pp. 293–306

4. Molecular-level understanding of support effects on the regenerability of Ru-based catalysts in the sulfur-poisoned methanation reaction

5. Influence of the support on sulfur poisoning and regeneration of Ru catalysts probed by sulfur K-edge X-ray absorption spectroscopy

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