Characterizing the solid hydrolysis product, UF4(H2O)2.5, generated from neat water reactions with UF4 at room temperature-Reference-Cited by-同舟云学术

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Characterizing the solid hydrolysis product, UF4(H2O)2.5, generated from neat water reactions with UF4 at room temperature

Published:2021 Issue:7 Volume:50 Page:2462-2471
ISSN:1477-9226
Container-title:Dalton Transactions
language:en
Short-container-title:Dalton Trans.

Author:

Christian Jonathan H.¹²³^ORCID,Klug Christopher A.⁴⁵³^ORCID,DeVore Michael¹²³^ORCID,Villa-Aleman Eliel¹²³^ORCID,Foley Bryan J.¹²³^ORCID,Groden Nicholas¹²³^ORCID,Baldwin A. Taylor¹²³^ORCID,Wellons Matthew S.¹²³^ORCID

Affiliation:

1. Savannah River National Laboratory

2. Aiken

3. USA

4. Naval Research Laboratory

5. Washington

Abstract

Anhydrous UF₄ stirred in water for 1–6 days forms UF₄(H₂O)_2.5 and a minor amount of uranyl fluoride. This hydrolysis results in morphological and spectroscopic changes.

Funder

Savannah River National Laboratory

Office of Environmental Management

Publisher

Royal Society of Chemistry (RSC)

Subject

Inorganic Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2021/DT/D0DT03944F

Reference46 articles.

1. Nuclear Forensic Science: Analysis of Nuclear Material Out of Regulatory Control

2. D. Féron , in Nuclear Corrosion Science and Engineering , ed. D. Féron , Woodhead Publishing , 2012 , pp. 31–56

3. Microscopy and spectroscopy of plutonium dioxide aging under ambient and near-ambient conditions

4. Characterizing the degradation of [(UO2F2)(H2O)]7 4H2O under humid conditions

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