Bragg coherent diffraction imaging with the CITIUS charge-integrating detector

Author:

Grimes MichaelORCID,Pauwels KristofORCID,Schülli Tobias U.,Martin Thierry,Fajardo PabloORCID,Douissard Paul-Antoine,Kocsis MenyhertORCID,Nishino HarukiORCID,Ozaki Kyosuke,Honjo YoshiakiORCID,Nishiyama Hiraki Toshiyuki,Joti YasumasaORCID,Hatsui TakakiORCID,Levi Mor,Rabkin Eugen,Leake Steven J.ORCID,Richard Marie-IngridORCID

Abstract

The CITIUS detector is a next-generation high-speed X-ray imaging detector. It has integrating-type pixels and is designed to show a consistent linear response at a frame rate of 17.4 kHz, which results in a saturation count rate of over 30 Mcps pixel−1 when operating at an acquisition duty cycle close to 100%, and up to 20 times higher with special extended acquisition modes. Here, its application for Bragg coherent diffraction imaging is demonstrated by taking advantage of the fourth-generation Extremely Brilliant Source of the European Synchrotron (ESRF-EBS, Grenoble, France). The CITIUS detector outperformed a photon-counting detector, similar spatial resolution being achieved (20 ± 6 nm versus 22 ± 9 nm) with greatly reduced acquisition times (23 s versus 200 s). It is also shown how the CITIUS detector can be expected to perform during dynamic Bragg coherent diffraction imaging measurements. Finally, the current limitations of the CITIUS detector and further optimizations for coherent imaging techniques are discussed.

Funder

H2020 European Research Council

Publisher

International Union of Crystallography (IUCr)

Subject

General Biochemistry, Genetics and Molecular Biology

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