Biomimetic tail-to-head terpene cyclizations using the resorcin[4]arene capsule catalyst
Author:
Funder
Swiss National Science Foundation - NCCR Catalysis
Novartis Universität Basel Excellence Scholarship
Publisher
Springer Science and Business Media LLC
Subject
General Biochemistry, Genetics and Molecular Biology
Link
https://www.nature.com/articles/s41596-023-00919-3.pdf
Reference61 articles.
1. Christianson, D. W. Structural and chemical biology of terpenoid cyclases. Chem. Rev. 117, 11570–11648 (2017).
2. Miller, D. J. & Allemann, R. K. Sesquiterpene synthases: passive catalysts or active players? Nat. Prod. Rep. 29, 60–71 (2012).
3. Pronin, S. V. & Shenvi, R. A. Synthesis of highly strained terpenes by non-stop tail-to-head polycyclization. Nat. Chem. 4, 915–920 (2012).
4. Lesburg, C. A., Zhai, G., Cane, D. E. & Christianson, D. W. Crystal structure of pentalenene synthase: mechanistic insights on terpenoid cyclization reactions in biology. Science 277, 1820 (1997).
5. Starks, C. M., Back, K., Chappell, J. & Noel, J. P. Structural basis for cyclic terpene biosynthesis by tobacco 5-epi-aristolochene synthase. Science 277, 1815 (1997).
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