Photon number statistics uncover the fluctuations in non-equilibrium lattice dynamics

Author:

Esposito Martina,Titimbo Kelvin,Zimmermann Klaus,Giusti Francesca,Randi Francesco,Boschetto Davide,Parmigiani Fulvio,Floreanini Roberto,Benatti Fabio,Fausti Daniele

Abstract

Abstract Fluctuations of the atomic positions are at the core of a large class of unusual material properties ranging from quantum para-electricity to high temperature superconductivity. Their measurement in solids is the subject of an intense scientific debate focused on seeking a methodology capable of establishing a direct link between the variance of the atomic displacements and experimentally measurable observables. Here we address this issue by means of non-equilibrium optical experiments performed in shot-noise-limited regime. The variance of the time-dependent atomic positions and momenta is directly mapped into the quantum fluctuations of the photon number of the scattered probing light. A fully quantum description of the non-linear interaction between photonic and phononic fields is benchmarked by unveiling the squeezing of thermal phonons in α-quartz.

Publisher

Springer Science and Business Media LLC

Subject

General Physics and Astronomy,General Biochemistry, Genetics and Molecular Biology,General Chemistry

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