Low-energy electronic structure in the unconventional charge-ordered state of ScV6Sn6

Author:

Kundu Asish K.,Huang XiongORCID,Seewald Eric,Ritz EthanORCID,Pakhira SantanuORCID,Zhang ShuaiORCID,Sun Dihao,Turkel SimonORCID,Shabani Sara,Yilmaz TurgutORCID,Vescovo Elio,Dean Cory R.ORCID,Johnston David C.,Valla TonicaORCID,Birol TuranORCID,Basov Dmitri N.ORCID,Fernandes Rafael M.ORCID,Pasupathy Abhay N.ORCID

Abstract

AbstractKagome vanadates AV3Sb5 display unusual low-temperature electronic properties including charge density waves (CDW), whose microscopic origin remains unsettled. Recently, CDW order has been discovered in a new material ScV6Sn6, providing an opportunity to explore whether the onset of CDW leads to unusual electronic properties. Here, we study this question using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy (STM). The ARPES measurements show minimal changes to the electronic structure after the onset of CDW. However, STM quasiparticle interference (QPI) measurements show strong dispersing features related to the CDW ordering vectors. A plausible explanation is the presence of a strong momentum-dependent scattering potential peaked at the CDW wavevector, associated with the existence of competing CDW instabilities. Our STM results further indicate that the bands most affected by the CDW are near vHS, analogous to the case of AV3Sb5 despite very different CDW wavevectors.

Funder

U.S. Department of Energy

Publisher

Springer Science and Business Media LLC

Reference70 articles.

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3. Li, H. et al. Observation of unconventional charge density wave without acoustic phonon anomaly in kagome superconductors AV3Sb5 (A = Rb, Cs). Phys. Rev. X 11, 031050 (2021).

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