Abstract
AbstractElemental tellurium is a small band-gap semiconductor, which is always p-doped due to the natural occurrence of vacancies. Its chiral non-centrosymmetric structure, characterized by helical chains arranged in a triangular lattice, and the presence of a spin-polarized Fermi surface, render tellurium a promising candidate for future applications. Here, we use a theoretical framework, appropriate for describing the corrections to conductivity from quantum interference effects, to show that a high-quality tellurium single crystal undergoes a quantum phase transition at low temperatures from an Anderson insulator to a correlated disordered metal at around 17 kbar. Such insulator-to-metal transition manifests itself in all measured physical quantities and their critical exponents are consistent with a scenario in which a pressure-induced Lifshitz transition shifts the Fermi level below the mobility edge, paving the way for a genuine Anderson-Mott transition. We conclude that previously puzzling quantum oscillation and transport measurements might be explained by a possible Anderson-Mott ground state and the observed phase transition.
Publisher
Springer Science and Business Media LLC
Reference49 articles.
1. Zhang, N. et al. Magnetotransport signatures of Weyl physics and discrete scale invariance in the elemental semiconductor tellurium. PNAS 117, 11337–11343 (2020).
2. Rikken, G. L. J. A. & Avarvari, N. Strong electrical magnetochiral anisotropy in tellurium. Phys. Rev. B 99, 245153 (2019).
3. Lin, S. et al. Tellurium as a high-performance elemental thermoelectric. Nat. Commun. 7, 10287 (2016).
4. Gao, Z., Liu, G. & Ren, J. High thermoelectric performance in two-dimensional tellurium: an ab initio study. ACS Appl. Mater. Interfaces 10, 40702–40709 (2018).
5. Qin, J. et al. Raman response and transport properties of tellurium atomic chains encapsulated in nanotubes. Nat. Electron. 3, 141–147 (2020).
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