A single probe for solvent dependent optical recognition of iron(II/III) and arsenite: discrimination between iron redox states with single crystal X-ray structure evidence

Author:

Das Jayanta,Ghosh Milan,Ghosh Biplab,Mandal Prasenjit,Maji Sangita,Das Debasis

Abstract

AbstractThe detection and discrimination of Fe2+ and Fe3+ ions have been investigated using a simple probe (L), produced by the condensation of ethylenediamine and 3-ethoxysalicyaldehyde. Single crystal X-ray structures demonstrate that L interacts with Fe2+ and Fe3+. In aqueous-DMSO media, the L recognises AsO2 by fluorescence and colorimetry techniques. The AsO2 aided PET inhibition and H-bond assisted chelation enhanced fluorescence (CHEF) boost fluorescence by 91-fold. The L can detect 0.354 ppb Fe2+, 0.22 ppb Fe3+ and 0.235 ppt AsO2.

Publisher

Springer Science and Business Media LLC

Subject

Multidisciplinary

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