Author:
Jena Anjan Kumar,Mallik Sameer Kumar,Sahu Mousam Charan,Sahoo Sandhyarani,Sahoo Ajit Kumar,Sharma Neha Kapila,Mohanty J.,Gupta Sanjeev K.,Ahuja Rajeev,Sahoo Satyaprakash
Abstract
AbstractStrain-mediated magnetism in 2D materials and dilute magnetic semiconductors hold multi-functional applications for future nano-electronics. Herein, First principles calculations are employed to study the influence of biaxial strain on the magnetic properties of Co-doped monolayer $$WS_2$$
W
S
2
. The non-magnetic $$WS_2$$
W
S
2
shows ferromagnetic signature upon Co doping due to spin polarization, which is further improved at low compressive (-2 %) and tensile (+2 %) strains. From the PDOS and spin density analysis, the opposite magnetic ordering is found to be favourable under the application of compressive and tensile strains. The double exchange interaction and p-d hybridization mechanisms make Co-doped $$WS_2$$
W
S
2
a potential host for magnetism. More importantly, the competition between exchange and crystal field splittings, i.e. ($$\Delta _{ex}>\Delta _{cfs}$$
Δ
ex
>
Δ
cfs
), of the Co-atom play pivotal roles in deciding the values of the magnetic moments under applied strain. Micromagnetic simulation reveals, the ferromagnetic behavior calculated from DFT exhibits low-field magnetic reversal (190 Oe). Moreover, the spins of Co-doped $$WS_2$$
W
S
2
are slightly tilted from the easy axis orientations showing slanted ferromagnetic hysteresis loop. The ferromagnetic nature of Co-doped $$WS_2$$
W
S
2
suppresses beyond $$\pm 2~\%$$
±
2
%
strain, which is reflected in terms of decrease in the coercivity in the micromagnetic simulation. The understanding of low-field magnetic reversal and spin orientations in Co-doped $$WS_2$$
W
S
2
may pave the way for next-generation spintronics and straintronics applications.
Publisher
Springer Science and Business Media LLC
Cited by
10 articles.
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