Demystifying the asymmetry-amplifying, autocatalytic behaviour of the Soai reaction through structural, mechanistic and computational studies
Author:
Publisher
Springer Science and Business Media LLC
Subject
General Chemical Engineering,General Chemistry
Link
http://www.nature.com/articles/s41557-020-0421-8.pdf
Reference47 articles.
1. Soai, K., Shibata, T., Morioka, H. & Choji, K. Asymmetric autocatalysis and amplification of enantiomeric excess of a chiral molecule. Nature 378, 767–768 (1995).
2. Soai, K., Kawasaki, T. & Matsumoto, A. Asymmetric autocatalysis of pyrimidyl alkanol and its application to the study on the origin of homochirality. Acc. Chem. Res. 47, 3643–3654 (2014).
3. Sato, I., Urabe, H., Ishiguro, S., Shibata, T. & Soai, K. Amplification of chirality from extremely low to greater than 99.5% e.e. by asymmetric autocatalysis. Angew. Chem. Int. Ed. 42, 315–317 (2003).
4. Soai, K. et al. Asymmetric synthesis of pyrimidyl alkanol without adding chiral substances by the addition of diisopropylzinc to pyrimidine-5-carbaldehyde in conjunction with asymmetric autocatalysis. Tetrahedron Asymmetry 14, 185–188 (2003).
5. Singleton, D. A. & Vo, L. K. Enantioselective synthesis without discrete optically active additives. J. Am. Chem. Soc. 124, 10010–10011 (2002).
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