1. Institute of Terrestrial Ecology, Department of Environmental Sciences, Swiss Federal Institute of Technology Zurich (ETHZ), ETH Zentrum, CHN, CH-8092 Zurich, Switzerland, Institute of Radiochemistry, Forschungszentrum Rossendorf eV, D-01314 Dresden, Germany, and Department of Physics and Astronomy, State University of New York (SUNY) Stony Brook, New York 11794-3800