Molecular Hydrogen Yields from the α-Self-Radiolysis of Nitric Acid Solutions Containing Plutonium or Americium

Author:

Gregson Colin R.1,Horne Gregory P.234ORCID,Orr Robin M.1ORCID,Pimblott Simon M.34,Sims Howard E.5,Taylor Robin J.1,Webb Kevin J.1

Affiliation:

1. Central Laboratory, National Nuclear Laboratory, Sellafield, Seascale, Cumbria CA20 1PG, U.K.

2. Dalton Cumbrian Facility, University of Manchester, Westlakes, Moor Row, Whitehaven CA24 3HA, U.K.

3. School of Chemistry, University of Manchester, Oxford Road, Manchester M13 9PL, U.K.

4. Idaho National Laboratory, 1955 N. Fremont Ave., Idaho Falls, Idaho 83415, United States

5. National Nuclear Laboratory, Culham Science Centre, Abingdon, Oxfordshire OX14 3DB, U.K.

Funder

Engineering and Physical Sciences Research Council

Nuclear Decommissioning Authority

FP7 Nuclear Fission, Safety and Radiation Protection

Dalton Cumbrian Facility, University of Manchester

Department of Energy and Climate Change, Government of the United Kingdom

Sellafield Ltd.

National Nuclear Laboratory, Government of the United Kingdom

Publisher

American Chemical Society (ACS)

Subject

Materials Chemistry,Surfaces, Coatings and Films,Physical and Theoretical Chemistry

Reference51 articles.

1. New activity coefficients of 0–100 per cent aqueous nitric acid

2. Inhibition of Radiolytic Molecular Hydrogen Formation by Quenching of Excited State Water

3. The Effect of Solutes on the Molecular Yields in the Radiolysis of Aqueous Solutions1

4. Yoshida, K.; Abe, H.; Yamane, Y.; Tashiro, S.; Muramatsu, K. Research on the State-of-the-Art of Accident Consequence Analysis Method for Non-Reactor Nuclear Facilities (1); Technical Report 2007-47 for Japan Atomic Energy Agency; Japan Atomic Energy Agency: Tokaimura, Japan, 2007.

5. May, R.; White, H. P. The Radiolysis of Nitric Acid in Highly Active Concentrates; Technical Report AERE-R-8646 for the Atomic Energy Research Establishment; Atomic Energy Research Establishment: Harwell, England, January 1977.

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