1. Environmental Science Department, Institute of Environmental and Natural Sciences, Lancaster University, LA1 4YQ, U.K., GKSS Research Centre, Max-Planck-Str. 1, D-21502 Geesthacht, Germany, Department of Environmental Chemistry, IIQAB-CSIC, Jordi Girona 18-24, Barcelona 08034, Catalunya, Spain, and Netherlands Institute for Sea Research, P.O. Box 59, NL-1790, Texel, The Netherlands