1. Aqueous Chemistry and Geochemistry Group, Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831-6110, H.H. Wills Physical Laboratory, Bristol University, Royal Fort, Tyndall Avenue, Bristol BS8 1TL, United Kingdom, and Institut Laue-Langevin, 6, rue Jules Horowitz BP 156-38042 Grenoble Cedex 9, France