Kinetic Study on Gas-Phase Beckmann Rearrangement of Cyclohexanone Oxime to ε-Caprolactam over a Silica-Supported Niobia Catalyst-Reference-Cited by-同舟云学术

Kinetic Study on Gas-Phase Beckmann Rearrangement of Cyclohexanone Oxime to ε-Caprolactam over a Silica-Supported Niobia Catalyst

Published:2016-01-29 Issue:5 Volume:55 Page:1202-1214
ISSN:0888-5885
Container-title:Industrial & Engineering Chemistry Research
language:en
Short-container-title:Ind. Eng. Chem. Res.

Author:

Maronna M. M.¹²³,Kruissink E. C.¹,Tinge J. T.¹,Agar D. W.²,Hoelderich W. F.⁴³

Affiliation:

1. DSM Chemical Technology R&D B.V., Urmonderbaan 22, 6167 RD Geleen, The Netherlands

2. Lehrstuhl für Technische Chemie B, TU Dortmund, Emil-Figge-Straße 66, 44227 Dortmund, Germany

3. Lehrstuhl für Technische Chemie und Heterogene Katalyse, RWTH Aachen, Worringerweg 1, 52074 Aachen, Germany

4. TCHK Consultancy, 67227 Frankenthal, Germany

Funder

Koninklijke DSM N.V.

Publisher

American Chemical Society (ACS)

Subject

Industrial and Manufacturing Engineering,General Chemical Engineering,General Chemistry

Link

https://pubs.acs.org/doi/pdf/10.1021/acs.iecr.5b04240

Reference49 articles.

1. Horn, P.; Grosskinsky, O.Verfahren zur kontinuierlichen Herstellung von epsilon-Caprolactam durch Beckmann’sche Umlagerung. Patent DE2845019A1, 1978.

2. Horn, P.; Grosskinsky, O.Process for the continuous manufacture of epsilon-caprolactam by the Beckmann conversion. U.S. Patent 4257950, 1981.

3. Smeets, T.; Lemmens, J.; Mostert, F.Continuous process for preparing caprolactam. Patent WO2004103964A1, 2004.

4. ϵ-Caprolactam: new by-product free synthesis routes

5. Modified Beta zeolites as catalysts for the Beckmann rearrangement of cyclohexanone oxime

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