1. Institute of Geological Sciences, School of Earth & Environment, University of Leeds, Leeds, LS2 9JT, U.K., Williamson Centre for Molecular Environmental Science, School of Earth, Atmospheric and Environmental Sciences, The University of Manchester, Manchester M13 9PL, U.K., Centre for Radiochemistry Research, and School of Earth, Atmospheric and Environmental Sciences, The University of Manchester, Manchester M13 9PL, U.K., and CLRC Daresbury Laboratory, Warrington, Cheshire WA4 4AD, U.K.