1. Research Centre for Radwaste and Decommissioning and Williamson Research Centre for Molecular Environmental Science, School of Earth, Atmospheric and Environmental Sciences, and Centre for Radiochemistry Research, School of Chemistry, The University of Manchester, Manchester, M13 9PL, U.K., Earth System Science Institute, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, U.K., and Karlsruhe Institute of Technology, Institut für Nukleare Entsorgung, D-76021-Karlsruhe, Germany