1. GKSS Research Centre Geesthacht, Institute for Coastal Research, Max-Planck Strasse 1, D-21502 Geesthacht, Germany; Institute of Ecology and Environmental Chemistry, University of Lüneburg, Scharmhorst Strasse 1, D-21335 Lueneburg, Germany; and LAVES, Philosophenweg 36/38, D-26121 Oldenburg, Germany