1. Soil Chemistry Group, Institute of Biogeochemistry and Pollutant Dynamics, Department of Environmental Sciences, ETH Zurich, CHN, Zurich CH-8092, Switzerland, Institut für Nukleare Entsorgung (INE), Forschungszentrum Karlsruhe, Karlsruhe D-76021, Germany, and National Cooperative for the Disposal of Radioactive Waste (Nagra), Wettingen CH-5430, Switzerland