1. Department of Environmental Science, Policy, and Management, Division of Ecosystem Sciences, University of California, Berkeley, California 94720-3114, Environmental Geochemistry Group, LGIT − Maison des Geosciences, Université J. Fourier and Centre National de la Recherche Scientifique (CNRS), B.P. 53, 38041 Grenoble Cedex 9, France, Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, and Department of Earth and Planetary Sciences, Harvard University, Cambridge,...