1. Department of Environmental Chemistry, IDAEA-CSIC, c/Jordi Girona 18-26, 08034 barcelona, Spain, Department of Water Quality Control, Technical University of Berlin, KF 4 Straβe des 17. Juni 135, D-10623, Berlin, Germany, Institucio Catalana de Reserca i Estudis Avanzats (ICREA), Barcelona, Spain, and Institut Català de Recerca de l’Aigua (ICRA), Parc Científic i Tecnológic de la, Universitat de Girona, Pic de Peguera, 15, 17003 Girona, Spain