1. Fundamental and Computational Sciences Directorate, Pacific Northwest National Laboratory, Richland, Washington 99352, Department of Civil and Environmental Engineering, University of Illinois at Urbana-Champaign, 205 N Mathews Ave, Urbana, Illinois 61801, Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99354, Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, Washington 99354, and Department of Geology, University...