Detailed Characterization of a Nanosecond-Lived Excited State: X-ray and Theoretical Investigation of the Quintet State in Photoexcited [Fe(terpy)2]2+

Author:

Vankó György1,Bordage Amélie1,Pápai Mátyás1,Haldrup Kristoffer2,Glatzel Pieter3,March Anne Marie4,Doumy Gilles4,Britz Alexander56,Galler Andreas5,Assefa Tadesse5,Cabaret Delphine7,Juhin Amélie7,van Driel Tim B.2,Kjær Kasper S.28,Dohn Asmus9,Møller Klaus B.9,Lemke Henrik T.10,Gallo Erik3,Rovezzi Mauro3,Németh Zoltán1,Rozsályi Emese1,Rozgonyi Tamás11,Uhlig Jens8,Sundström Villy8,Nielsen Martin M.2,Young Linda4,Southworth Stephen H.4,Bressler Christian56,Gawelda Wojciech5

Affiliation:

1. Wigner Research Centre for Physics, Hungarian Academy Sciences, P.O.B. 49., H-1525 Budapest, Hungary

2. Centre for Molecular Movies, Technical University of Denmark, Department of Physics, DK-2800 Kgs. Lyngby, Denmark

3. European Synchrotron Radiation Facility (ESRF), CS40220, Grenoble 38043 Cedex 9, France

4. X-ray Science Division, Advanced Photon Source, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, Illinois 60439, United States

5. European XFEL, Albert-Einstein-Ring 19, D-22761 Hamburg, Germany

6. The Hamburg Centre for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany

7. Institut de Minéralogie, de Physique des Matériaux, et de Cosmochimie (IMPMC), Sorbonne Universités - UPMC Univ. Paris 06, UMR CNRS 7590, Muséum National d’Histoire Naturelle, UR IRD 206, 4 Place Jussieu, F-75005 Paris, France

8. Department of Chemical Physics, Lund University, Box 124, 22100 Lund, Sweden

9. Centre for Molecular Movies, Technical University of Denmark, Department of Chemistry, DK-2800 Kgs. Lyngby, Denmark

10. SLAC National Accelerator Laboratory, Linac Coherent Light Source, Menlo Park, California 94025, United States

11. Research Centre for Natural Sciences, Hungarian Academy of Sciences, P.O. Box 286, H-1519 Budapest, Hungary

Funder

European Research Council

Danish National Research Foundation

Magyar Tudományos Akadémia

Deutsche Forschungsgemeinschaft

Knut och Alice Wallenbergs Stiftelse

Ministère de l'Enseignement Supérieur et de la Recherche

Ministère des Affaires Étrangères

Cluster of Research Infrastructures for Synergies in Physics

Hungarian and French Intergovernmental Science and Technology Cooperation Program

Publisher

American Chemical Society (ACS)

Subject

Surfaces, Coatings and Films,Physical and Theoretical Chemistry,General Energy,Electronic, Optical and Magnetic Materials

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