Uncovering the Origin of the Emitting States in Bi3+-Activated CaMO3 (M = Zr, Sn, Ti) Perovskites: Metal-To-Metal Charge Transfer Versus s

Uncovering the Origin of the Emitting States in Bi3+-Activated CaMO3 (M = Zr, Sn, Ti) Perovskites: Metal-To-Metal Charge Transfer Versus s–p Transitions

Published:2019-05-15 Issue:23 Volume:123 Page:14677-14688
ISSN:1932-7447
Container-title:The Journal of Physical Chemistry C
language:en
Short-container-title:J. Phys. Chem. C

Author:

Back Michele¹^ORCID,Ueda Jumpei¹^ORCID,Xu Jian¹^ORCID,Asami Kazuki¹^ORCID,Amidani Lucia²³^ORCID,Trave Enrico⁴^ORCID,Tanabe Setsuhisa¹^ORCID

Affiliation:

1. Graduate School of Human and Environmental Studies, Kyoto University, Kyoto 606-8501, Japan

2. Rossendorf Beamline at ESRF—The European Synchrotron, CS40220, 38043 Grenoble Cedex 9, France

3. Helmholtz-Zentrum Dresden-Rossendorf, Institute of Resource Ecology, P.O. Box 510119, 01314 Dresden, Germany

4. Department of Molecular Sciences and Nanosystems, Università Ca’ Foscari Venezia, Via Torino 155, 30172 Mestre-Venezia, Italy

Funder

Institute for Molecular Science

Japan Society for the Promotion of Science

H2020 European Research Council

Publisher

American Chemical Society (ACS)

Subject

Surfaces, Coatings and Films,Physical and Theoretical Chemistry,General Energy,Electronic, Optical and Magnetic Materials

Link

https://pubs.acs.org/doi/pdf/10.1021/acs.jpcc.9b03940

Reference77 articles.

1. H2or O2Evolution from Aqueous Solutions on Layered Oxide Photocatalysts Consisting of Bi3+with 6s2Configuration and d0Transition Metal Ions

2. Lead Bismuth Oxyhalides PbBiO2X (X = Cl, Br) as Visible-Light-Responsive Photocatalysts for Water Oxidation: Role of Lone-Pair Electrons in Valence Band Engineering

3. Valence Band Engineering of Layered Bismuth Oxyhalides toward Stable Visible-Light Water Splitting: Madelung Site Potential Analysis

4. Enhancement of the chemical stability in confined δ-Bi2O3

5. Ferroelectricity in Ordered Perovskite BaBi0.53+(Bi0.25+Nb0.35+)O3 with Bi3+:6s2 Lone Pair at the B-site

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