1. Institute of Ecological Chemistry, Helmholtz Zentrum Muenchen, German Research Center for Environmental Health, Ingolstaedter Landstrasse 1, D-85764 Neuherberg, Germany, Bruker Daltonics, Fahrenheitstrasse 4, D-28359 Bremen, Germany, Alfred-Wegener-Institut für Polar- and Meeresforschung, Am Handelshafen 12, 27570 Bremerhaven, Germany, and School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, Georgia 30332