Experimental and Computational Investigation of Acetic Acid Deoxygenation over Oxophilic Molybdenum Carbide: Surface Chemistry and Active Site Identity

Author:

Schaidle Joshua A.1,Blackburn Jeffrey1,Farberow Carrie A.1,Nash Connor1,Steirer K. Xerxes1,Clark Jared1,Robichaud David J.1,Ruddy Daniel A.1

Affiliation:

1. National Bioenergy Center, ‡Chemistry and Nanoscience Center, and #Materials Science Center, National Renewable Energy Laboratory, Golden, Colorado 80401, United States

Funder

Office of Energy Efficiency and Renewable Energy

Laboratory Directed Research and Development

Publisher

American Chemical Society (ACS)

Subject

Catalysis,General Chemistry

Reference70 articles.

1. Multi-Year Program Plan;U.S. Department of Energy Bioenergy Technologies Office:Washington, DC, 2015. See:http://www.energy.gov/sites/prod/files/2015/04/f22/mypp_beto_march2015.pdf.

2. Dutta, A.; Sahir, A.; Tan, E.; Humbird, D.; Snowden-Swan, L. J.; Meyer, P.; Ross, J.; Sexton, D.; Yap, R.; Lukas, J.Process Design and Economics for the Conversion of Lignocellulosic Biomass to Hydrocarbon Fuels: Thermochemical Research Pathways with In Situ and Ex Situ Upgrading of Fast Pyrolysis Vapors, NREL/TP-5100–62455,National Renewable Energy Laboratory (NREL):Golden, CO, 2015.

3. Biddy, M.; Dutta, A.; Jones, S.; Meyer, A.Ex-situ Catalytic Fast Pyrolysis Technology Pathway, NREL/TP-5100–58050,National Renewable Energy Laboratory (NREL):Golden, CO, 2013.

4. Conceptual Process Design and Techno-Economic Assessment of Ex Situ Catalytic Fast Pyrolysis of Biomass: A Fixed Bed Reactor Implementation Scenario for Future Feasibility

5. Recent advances in heterogeneous catalysts for bio-oil upgrading via “ex situ catalytic fast pyrolysis”: catalyst development through the study of model compounds

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