1. Eawag, Swiss Federal Institute of Aquatic Science and Technology, Ueberlandstrasse 133, CH-8600 Duebendorf, Switzerland, Soil Chemistry Group, Institute of Biogeochemistry and Pollutant Dynamics, ETH Zurich, CHN, CH-8092 Zurich, Switzerland, Institute of Radiochemistry, FZD, Dresden, Germany, and Rossendorf Beamline, European Synchrotron Radiation Facility, Grenoble, France