Phosphine-Mediated [4 + 2] Annulation of Bis(enones): A Lewis Base Catalyzed “Mock Diels−Alder” Reaction
Author:
Affiliation:
1. Chemical Research and Development, Pfizer Global Research and Development, Eastern Point Road, P.O. Box 8013, Groton, Connecticut 06340-8013
Publisher
American Chemical Society (ACS)
Subject
Organic Chemistry,Physical and Theoretical Chemistry,Biochemistry
Link
https://pubs.acs.org/doi/pdf/10.1021/ol049392v
Reference28 articles.
1. The Diels-Alder Reaction in Total Synthesis
2. Catalytic Enantioselective Diels-Alder Reactions: Methods, Mechanistic Fundamentals, Pathways, and Applications
3. Highly Enantioselective Inverse-Electron-Demand Hetero-DielsâAlder Reactions of α,β-Unsaturated Aldehydes This work was supported by the NIH (GM-59316), with additional support from the Schweizerischer Nationalfonds zur Förderung der wissenschaftlichen Forschung (postdoctoral fellowship to K.G.), and the National Science Foundation (predoctoral fellowship to D.E.C.). We are grateful to Dr. R. Staples for carrying out the X-ray crystal structure analysis of 1.
4. Novel cyclization reactions on transition metal templates. The catalysis of intramolecular [4+2] cycloadditions by low-valent rhodium complexes
5. On the asymmetric rh(I) catalyzed [4+2] cycloisomerization reaction. Electronic and torsional ligand control of absolute stereoselection.
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