Abstract
The A
2
Σ+ -X
2
II
1
(a) absorption system of the NCO free radical has been re-investigated with higher resolving power than in the earlier work of Dixon (i960). Particular emphasis has been directed to the rotational analyses of bands involving the three vibronic levels, μ
2
Σ
(+)
,
2
Δ
i
-(a) and k
2
Σ
(-)
, associated with the first level of the bending vibration in the ground state. A misassignment in the earlier work has been corrected and a new value for the Renner parameter determined, namely ε = -0.144 ± 0.001. This revised value removes the discrepancy noted in the earlier electron resonance results.
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