Self-assembled platinum-tungsten carbide (Pt-WC)/multi-walled carbon nanotubes (MWCNTs) electrocatalysts for ethanol electro-oxidation in acid medium

Author:

Ai Tianyu1,Zhang Yi1,Lu Jinlin1,Yin Yansheng1

Affiliation:

1. Research Center for Corrosion and Erosion Process Control of Equipment and Material in Marine Harsh Environment, Guangzhou Maritime University, Guangzhou, Guangdong, 510725, China

Abstract

The design of a high-performance, durable and low-cost catalyst for direct ethanol fuel cells (DEFCs) applications is an eternal pursuit for researchers in the materials field. In this work, a kind of novel platinum-tungsten carbide (Pt-WC)/multi-walled carbon nanotubes (MWCNTs) electrocatalyst with different WC loadingsis prepared by self-assembly technology for ethanol oxidation reaction (EOR). The electrochemical performance and stability of Pt-WC/MWCNTs electrocatalysts toward EOR are investigated by cyclic voltammetry and chronoamperometry. The mass activity of Pt-WC0.15/MWCNTs electrocatalyst for EOR is 581.94 mA mg-1Pt, which is 1.33 times higher than that of commercial Pt/C (ETEK). The significant enhancement can be attributed to the more exposed active sites and the synergistic effect between Pt and WC. The Pt-WCx/MWCNTs are a kind of excellent and effective electrocatalyst for EOR, which has a broad application prospect in fuel cells.

Publisher

American Scientific Publishers

Subject

General Materials Science

Reference37 articles.

1. Ethanol oxidation on a carbon-supported Pt75Sn25 electrocatalyst prepared by reduction with formic acid: Effect of thermal treatment.;Colmati;Applied Catalysis B: Environmental,2007

2. Electrocatalytic activity and stability of Pt supported on Sb-doped SnO2 nanoparticles for direct alcohol fuel cells.;Lee;Journal of Catalysis,2008

3. Hydrogen gas-assisted synthesis of worm-like PtMo wavy nanowires as efficient catalysts for the methanol oxidation reaction.;Lu;Journal of Materials Chemistry A,2016

4. Synthesis and catalytic property of PtSn/C toward the ethanol oxidation reaction.;Su;International Journal of Electrochemical Science,2012

5. Electrochemical and in situ FTIR study of the ethanol oxidation reaction on PtMo/C nanomaterials in alkaline media.;Pech-Rodríguez;Applied Catalysis B: Environmental,2017

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