Fabrication and Optical Performance of Mo1-xWxS2 Monolayer with Different Composition Ranges via One-Step Chemical Vapor Deposition Approach

Author:

Chen Fei1,Jiang Xia2,Zheng Xin1,Lu Bin3,Deng Tingting4

Affiliation:

1. College of Materials and Environmental Engineering, Hangzhou Dianzi University, Hangzhou 310018, PR China

2. School of Electronics and Information Engineering, Hangzhou Dianzi University, Hangzhou 310018, PR China

3. Institute of Advanced Magnetic Materials, College of Materials and Environmental Engineering, Hangzhou Dianzi University, Hangzhou 310018, PR China

4. School of Physics and Optoelectronic Engineering, Foshan University, Foshan 528225, PR China

Abstract

Fabrication of 2D TMDCs with variable bandgap can supply a prospective platform for the multi-functional applications in optoelectronics. Here, we present a one-step CVD strategy for realization of 2D Mo1-xWxS2 flakes with different x ranges through adjusting growth temperature. Detailed Raman and photoluminescence spectra/mappings have elucidated that as-produced Mo1-xWxS2 alloys exhibit significant compositiondependent structural and optical modulation. The variation of Mo1-xWxS2 alloy with diverse composition ranges has discussed based on the effect of growth temperature on the evaporation and interdiffusion of Mo/W atoms. The present results will provide a favorable guidance for the controllable fabrication of other 2D TMDC alloys, providing prospective materials for functional optoelectronics.

Publisher

American Scientific Publishers

Subject

Electrical and Electronic Engineering,Electronic, Optical and Magnetic Materials

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