On-Line Measurements of the Volatilization of Ruthenium in a Vitrification Process

Author:

Odoj R.,Schwitz M.

Abstract

ABSTRACTThe studies were performed using Ru–103 as a tracer. The volatilization of Ru from ruthenium containing liquids, like HAW-solutions, is about 15%. A chemical denitration of these solutions with HCHO or HCOOH reduces the volatilization to about 2%. Additional catalytic reduction with Fe-powder lowers the volatilization to about 4 ‰. The carry over of Ru seems to depend on the aerosol production rate and not the vapor pressure. Only RuO2 could be detected in the off-gas.

Publisher

Springer Science and Business Media LLC

Subject

General Engineering

Reference4 articles.

1. Effect of Denitration on Ruthenium Volatilization

2. “ProzeBverlauf und Reaktionsmcdell der Denitrierung von HLLW nit HCHO”;Odoj;Jül-Bericht,1982

3. “Nitrato and Nitro Complexes of Nitrosylruthenium”;Fletcher;J. Inorg. Chem.,1955

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