Author:
Shi Shunli,Yu Ying,Zhang Bingzhen,Zhong Yicheng,Wang Lei,Wang Shuhua,Ding Shunmin,Chen Chao
Abstract
The development of efficient heterogeneous catalysts for one-pot tandem/cascade synthesis of imines remains meaningful and challenging. Herein, we constructed an Au/MOF catalyst featured hollow and double MOF shell nanostructure. Owing to its structural merits and acid-basic nature, the as-synthesized Void|(Au)ZIF-8|ZIF-8 catalyst exhibited an enhanced synergistically catalytic performance for tandem catalytic synthesis of imines from benzyl alcohol and aniline under air atmosphere and solvent-free condition. Its 170.16 h−1 of turnover frequency (TOF) was 2.5 times higher than that of the reported catalyst with the highest TOF value.
Funder
National Natural Science Foundation of China
Natural Science Foundation of Jiangxi Province
Cited by
8 articles.
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