Analysis of Ozone Production Reaction Rate and Partial Discharge Power in a Dielectric-Barrier Acrylic Chamber with 60 Hz High-Voltage Electrodes: CFD and Experimental Investigations

Abstract

We present a synergistic investigation into ozone production dynamics within a high-voltage reaction chamber operating from 1.75 kV to 10 kV, at 60 Hz. The output ozone concentration dependence on a 60 Hz root mean square high-voltage for an air input pressure of 0.1 bar was measured using an ultraviolet-based sensor. A finite-element numerical model of the reaction chamber was developed and used for obtaining the reaction rate for the generated ozone for each level of input voltage and the internal distribution of the gas vector velocity field and ozone concentration. An expression to estimate the ozone reaction rates from the measured ozone concentrations was also derived. It was then compared and validated using the developed computational model. Therefore, in this work, a formula is proposed to estimate the ozone production by providing the experimental reaction rates. The other objective is to analyze the hysteresis phenomena observed in the partial discharges’ levels in the reaction chamber and in the output ozone concentration. Finally, we establish a connection between the total power of partial discharges and the consequent ozone production, clarifying the role of cumulative partial discharges’ power levels in governing the resultant output ozone concentration.