Rapid Antibiotic Adsorption from Water Using MCM-41-Based Material

Author:

Chen Jie1,Yang Yao2,Yao Yuanyuan1,Huang Zhujian2ORCID,Xu Qiaoling2,He Liping1,Gong Beini2

Affiliation:

1. CCCC Fourth Harbor Engineering Institute Co., Ltd., Guangzhou 510230, China

2. Guangdong Provincial Key Laboratory of Agricultural & Rural Pollution Abatement and Environmental Safety, College of Natural Resources and Environment, South China Agricultural University, Guangzhou 510642, China

Abstract

The contamination of antibiotics in the environment has raised serious concerns, impacting both human life and ecosystems. This has led to a growing focus on the development of cost-effective and environmentally friendly adsorbent materials. Mesoporous molecular sieve MCM-41, known for its strong adsorption capacity, low cost, and efficient regenerative properties, holds significant promise for addressing this issue. In this study, we investigated the adsorption behavior of demolded MCM-41 materials in relation to tetracycline, doxycycline, and levofloxacin at different temperatures and pH levels. Our experiments encompassed the adsorption of these three common antibiotics, revealing that a neutral or weakly acidic pH environment promoted adsorption, whereas alkaline conditions hindered it. Utilizing the equilibrium isotherm model, we determined the theoretical maximum adsorption capacities for tetracycline (TC), doxycycline (DOX), and levofloxacin (LFX) as 73.41, 144.83, and 33.67 mg g−1, respectively. These findings underscore the significant potential of MCM-41 in mitigating antibiotic wastewater contamination.

Funder

Key-Area Research and Development Program of Guangdong Province

Natural Science Foundation of Guangdong Province

National Natural Science Foundation of China

Beijing Zhongkebaice Technology Service Co., Ltd.

Publisher

MDPI AG

Subject

Water Science and Technology,Aquatic Science,Geography, Planning and Development,Biochemistry

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